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If you have JAVA experience, C# would be easy for you to learn. Contrary to what some other people are answering, ASP.NET does NOT need to run on a Windows server and all the necessary components to get started learning are free.
If you're working on an existing site, it's probably going to be a lot easier for you to just continue on with PHP rather than trying to recreate it in a language that's new to you.
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